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Delete /home/username/.wine directory
Then in terminal run: winecfg
Literally does what you want! You WILL lose anything installed in default prefix, like games/apps, if you didn’t make separate prefixes for them.
Edit: Just saw you’re running chromebook, the locations might differ. My notes were for Debian/Ubuntu & their flavors.
LTSC is the route I took as well for awhile. But went back to retail because I wanted to play Game Pass and there were some weird things going on. But it was great for my cheap homemade NAS.
that is… until I switched both computers to Linux last year.
But completely agree - if you need/want to stay in Windows, LTSC was very clean.